2023
DOI: 10.1039/d2cp05447g
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Nano-droplet jumping due to surface wettability variation: molecular modeling approach

Abstract: The effect of substrate hydrophobicity on the dynamics of water nano-droplets is computationally studied utilizing the molecular dynamics method. It is observed that the droplet moves upward by increasing the...

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Cited by 3 publications
(2 citation statements)
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“…Some studies have successfully tuned the jumping behaviors of the droplets by adjusting the parameters such as the number and size, 16 or by utilizing heterogeneous droplets. 17 A more commonly implemented strategy is to modulate the surface properties or morphology, such as surface wettability, 18 honeycomb bionic superhydrophobic surfaces, 19 mixed-wettability superhydrophobic surfaces, 20 micro-or nanoarray decorated surfaces, [21][22][23] hierarchical surface structures, [24][25][26] macrotexures, 15,27,28 etc. These microstructures, nature inspired or artificial, in general are designed to reduce the adhesion when the merged droplet detaches from the surface.…”
Section: Introductionmentioning
confidence: 99%
“…Some studies have successfully tuned the jumping behaviors of the droplets by adjusting the parameters such as the number and size, 16 or by utilizing heterogeneous droplets. 17 A more commonly implemented strategy is to modulate the surface properties or morphology, such as surface wettability, 18 honeycomb bionic superhydrophobic surfaces, 19 mixed-wettability superhydrophobic surfaces, 20 micro-or nanoarray decorated surfaces, [21][22][23] hierarchical surface structures, [24][25][26] macrotexures, 15,27,28 etc. These microstructures, nature inspired or artificial, in general are designed to reduce the adhesion when the merged droplet detaches from the surface.…”
Section: Introductionmentioning
confidence: 99%
“…Using the single-shot multiframe methodology developed here, we succeeded in directly observing the entire melting/jumping processes of the same NP at ∼12 nm resolution and quantitatively describing such behaviors with the correction algorithm. Regarding the jumping process, several mechanisms have been proposed in the past years: (i) plasma-induced shockwave; , (ii) dewetting-induced detachment; , and (iii) coalescence-induced jumping. The detachment and jumping of the NPs induced by the plasma-associated shockwave require the high-power short-pulse laser to trigger the process. According to a model of the nanosecond-laser-induced heat transfer between the Au NP and the SiN film (Figure S8), the simulation suggested that the temperature of the Au NP became ∼1400 K at a fluence of 36 mJ/cm 2 (Figure S9).…”
mentioning
confidence: 99%