Multipolar Conjugated Polymer Framework Derived Ionic Sieves via Electronic Modulation for Long‐Life All‐Solid‐State Li Batteries
Xue Yang,
Long Fang,
Jing Li
et al.
Abstract:Here, we build a tunable multipolar conjugated polymer framework platform via pore wall chemistry to probe the role of electronic structure engineering in improving the Li+ conduction by theoretical studies. Guided by theoretical prediction, we develop a new cyano‐vinylene‐linked multipolar polymer framework namely CNF‐COF, acting as efficient ion sieves to modify polymer electrolytes for long‐lifespan all‐solid‐state (ASS) Li metal batteries. The cyano and fluorine groups dual‐decoration in CNF‐COF favorably… Show more
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