The growing concern over low-frequency noise pollution
resulting
from global industrialization has posed substantial challenges in
noise attenuation. However, conventional acoustic metamaterials, with
fixed geometries, offer limited flexibility in the frequency range
adjustment once constructed. This research unveiled the promising
potential of ionic electroactive polymers, particularly ionic polymer–metal
composites (IPMCs), as a superior candidate to design tunable acoustic
metamaterial due to its bidirectional energy conversion capabilities.
The previously perceived limitations of the IPMC, including slow reaction
and high energy expenditure, owning to its inherent sluggish intermediary
ionic mass transport process, were astutely leveraged to expedite
the attenuation of low-frequency sound energy. Both our experimental
and simulation results elucidated that the IPMC can generate voltage
potentials in response to acoustic pressure at frequencies significantly
higher than those previously established. In addition, the peak absorption
frequency can be effectively shifted by up to 45.7% with the application
of a 4 V voltage. By further integration with a microperforated panel
(MPP) structure, the developed metamaterial absorbers can achieve
complete sound absorption, which was continuously tunable under minimal
voltage stimulation across a wide frequency spectrum. In addition,
a microslit structure IPMC metamaterial absorber was designed to realize
modulation of the perforation rate, and the absorption peak can be
shifted by up to 79.2%. These findings signify a pioneering application
of ionic intelligent materials and may pave the way for further innovations
of tunable low-frequency acoustic structures, ultimately advancing
the pragmatic deployment of both soft intelligent materials and acoustic
metamaterials.