1996
DOI: 10.1021/jp9536559
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Monte Carlo Simulation of Range and Energy Deposition by Electrons in Gaseous and Liquid Water

Abstract: A stochastic simulation method employing suitable experimentally based cross sections has been developed for probing the spatial distribution of energy loss and the trajectory of 100 eV to 1 MeV electrons in gaseous and liquid water. Elastic collisions and large-energy-loss inelastic collisions strongly influence the passage of electrons such that the separation between the initial and final (E = 25 eV) position is considerably smaller than the path length. At all energies, the mean axial and the mean radial p… Show more

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Cited by 130 publications
(147 citation statements)
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“…Many chemical reactions take place as well; they are also important for estimates of the DNA damage since they define the agents interacting with the DNA. Again, this aspect has attracted plenty of attention of Monte Carlo simulations adepts [5] who, using various SDCS of ionization (including the effects of the medium [6][7][8][9]), trace the electrons and other species through the medium up to their interaction with the DNA. We developed an approach to calculations that can be done on this scale without using Monte Carlo simulations [10,11].…”
Section: Propagation Of Secondary Electrons and Dna Damagementioning
confidence: 99%
“…Many chemical reactions take place as well; they are also important for estimates of the DNA damage since they define the agents interacting with the DNA. Again, this aspect has attracted plenty of attention of Monte Carlo simulations adepts [5] who, using various SDCS of ionization (including the effects of the medium [6][7][8][9]), trace the electrons and other species through the medium up to their interaction with the DNA. We developed an approach to calculations that can be done on this scale without using Monte Carlo simulations [10,11].…”
Section: Propagation Of Secondary Electrons and Dna Damagementioning
confidence: 99%
“…Secondary electrons, whose distribution lies mostly below 20 eV, are the most abundant of these secondary species. 3 Whether created by ionization of DNA or surrounding molecules, such as H 2 O, secondary electrons can interact with DNA, break chemical bonds, and create harmful radicals and ions. Thus, they account for a large portion of the direct and indirect effects of ionizing radiation on DNA.…”
Section: Introductionmentioning
confidence: 99%
“…and 500 eV is very close in all the three cases 65 , and hence the different kinetic energy could arguably explain the significant change of hundreds of seconds in the appearance of the desorption peaks as shown in Figure 4. More realistically, the observed trend can be rationalised in three ways:…”
Section: Methodsmentioning
confidence: 85%
“…at a certain depth within the ice film where it loses most of its energy 65 . thickness of the slab is 44.5 nm.…”
mentioning
confidence: 99%