Abstract:Aqueous zinc-iodine batteries (AZIBs) with high theoretical capacities, intrinsic safety, and low cost have been extensively explored as one of next-generation energy storage devices. Nevertheless, in the presence of aqueous electrolytes, AZIBs suffer severe metal corrosion, dendrite growth, and polyiodide shuttling, leading to fast capacity degradation. Here, we report a molecule chemistry strategy by making use of tris(2-cyanoethyl) borate to form a gradient solid electrolyte interface, which dynamically ada… Show more
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