2001
DOI: 10.1515/zna-2001-0606
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Molecular Dynamics Study on the Adsorption Selectivity for Negative Elements in Aluminosilicates

Abstract: For the pyrochemical reprocessing o f spent metallic nuclear fuels in molten salt baths it is important to investigate the adsorption selectivity o f cations in aluminosilicates. A molecular dynamics simulation has been performed on sodalite and zeolite with exchangeable monovalent and multivalent cationic fission products at 673 K in order to calculate their self-diffusion coefficients in the aluminosilicate framework and estimate the selectivity o f the exchangeable cations. The results enables us to conclud… Show more

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