2021
DOI: 10.1021/acs.energyfuels.1c01671
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Molecular Characterization of Fossil and Alternative Fuels Using Electrospray Ionization Fourier Transform Ion Cyclotron Resonance Mass Spectrometry: Recent Advances and Perspectives

Abstract: Molecular composition analysis of petroleum and alternative fuels has been considered as one of the greatest challenges in analytical chemistry. The rapid development of Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS) has provided an opportunity to solve this problem. High mass resolution power and mass accuracy enable the separation of isobaric compounds in a complex mixture and assignment of their molecular composition. The combination of electrospray ionization (ESI) with FT-ICR MS a… Show more

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Cited by 30 publications
(18 citation statements)
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“…Our environment is now getting polluted due to the emission of greenhouse gases from different sources like industries and automobiles engines. , The heavy vehicles that consume fossil fuels are considered to be one of the major contributors to the emission of poisonous gases like CO, CO 2 , SO 2 , and NO. , Because of this, the environmental pollution laws have been imposed to restrict such damage to our environment. In this regard, alternative energy sources like H 2 gas, biogas, and biofuels are greener fuels that can protect our environment from climate change. Recent progress in the field of energy sectors considers alcohols such as methanol (CH 3 OH) and ethanol (C 2 H 5 OH) as alternative sources of energy. Both CH 3 OH and C 2 H 5 OH are beneficial because of their good electrochemical activity, their availability, and their biodegradability. , Most importantly, both CH 3 OH and C 2 H 5 OH do not need much special care for transportation as it is needed for H 2 gas. , Apart from this specific characteristic, the energy density of CH 3 OH and C 2 H 5 OH are also compatible with H 2 fuel, for which it can take the market value. Due to such beneficial factors, researchers across the world are searching for new catalysts that can boost the electrochemical oxidation of CH 3 OH and C 2 H 5 OH for use as a material for liquid fuel cells. , …”
Section: Introductionmentioning
confidence: 99%
“…Our environment is now getting polluted due to the emission of greenhouse gases from different sources like industries and automobiles engines. , The heavy vehicles that consume fossil fuels are considered to be one of the major contributors to the emission of poisonous gases like CO, CO 2 , SO 2 , and NO. , Because of this, the environmental pollution laws have been imposed to restrict such damage to our environment. In this regard, alternative energy sources like H 2 gas, biogas, and biofuels are greener fuels that can protect our environment from climate change. Recent progress in the field of energy sectors considers alcohols such as methanol (CH 3 OH) and ethanol (C 2 H 5 OH) as alternative sources of energy. Both CH 3 OH and C 2 H 5 OH are beneficial because of their good electrochemical activity, their availability, and their biodegradability. , Most importantly, both CH 3 OH and C 2 H 5 OH do not need much special care for transportation as it is needed for H 2 gas. , Apart from this specific characteristic, the energy density of CH 3 OH and C 2 H 5 OH are also compatible with H 2 fuel, for which it can take the market value. Due to such beneficial factors, researchers across the world are searching for new catalysts that can boost the electrochemical oxidation of CH 3 OH and C 2 H 5 OH for use as a material for liquid fuel cells. , …”
Section: Introductionmentioning
confidence: 99%
“…Additionally, considerable uncertainties exist in selecting one proper formula from the multiple formula assignments. To alleviate this problem, the formula screening can be conducted according to following rules (Liu et al, 2015;Shi et al, 2021;Vetere and Schrader, 2017). In most cases, CHO components were more reliable than CHON components (Herzsprung et al, 2014(Herzsprung et al, , 2015.…”
Section: Fourier Transform Ion Cyclotron Resonance Mass Spectrometry ...mentioning
confidence: 99%
“…The author highlighted the unparalleled high mass resolution power of MS and the need to work with various techniques, including separations, different ionization methods, ion dissociation/multidimensional MS, and hyphened separation techniques. Shi and co-workers from China University of Petroleum (Beijing) 41 provided a historical (vertical) perspective of the development of MS techniques, with a special focus on electrospray ionization (ESI) for the detection of polar compounds in petroleum.…”
Section: ■ Ft-icr Ms Overviewmentioning
confidence: 99%