Abstract:Modelling of series reactions was performed for core–shell catalysts. Mathematical solutions of concentrations inside the pellets were derived from reaction–diffusion equations considering inert‐core thickness (ξc) for first‐order kinetics. Transient behaviours of catalytic reactors containing core–shell pellets were predicted, assuming pseudo‐steady state approximation. In a batch reactor, the removal rate of reactants increased with increasing Thiele modulus and decreasing ξc in the order of sphere > cylinde… Show more
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