Facing serious environmental degradation and its resulting of climate warming, how to conserve energy and reduce emissions becomes a serious issue for government supervisors and modern vehicle enterprises. Reducing the mass of a vehicle is one of the most effective ways to reduce emissions and improve fuel utilization, essential to persist the low-carbon and sustainable-development bases in industrial production processes. When it comes to the selection of lightweight material for a car body in the processes of vehicle production, it is essential to comprehensively evaluate multiple relevant attributes in order to select the optimal material from several alternatives. us, it can be seen as a multicriterion decision-making (MCDM) problem. However, it is difficult to consider both the uncertainty of the expert's preference and the imprecision of the attribute estimate. Considering this, this paper uses the method integrating grey relational analysis (GRA) with analytic hierarchy process (AHP) to solve the problem of lightweight material selection for a car body. e AHP method is used to determine the weight of each attribute, and the GRA method is to select the optimal material among several alternatives. Finally, a case study is applied to verify the practicability of the proposed approach. e result shows that the proposed multicriterion decision method provides a precise and objective foundation for making decisions about the material selection issue.