“…Featuring broad operation bandwidths, low power consumption, and potentially reduced cost, all-optical signal processing based on nonlinear photonic devices has provided a competitive solution to realize ultrafast signal processing. [1][2][3][4][5][6][7] As the key building blocks for implementing nonlinear photonic devices, advanced optical materials with superior nonlinear properties have been widely investigated. Recently, two-dimensional (2D) layered materials such as graphene [8,9], graphene oxide (GO) [10][11][12][13][14], transition metal dichalcogenides (TMDCs) [15][16][17], and black phosphorus (BP) [18][19][20] have attracted significant interest with their remarkable optical properties, such as ultrahigh Kerr optical nonlinearities, strong nonlinear absorption, significant material anisotropy, and layer-dependent material properties.…”