We have performed zero-field and longitudinal field muon spin experiments on single crystals of the Kondo lattice compound CePt 2 Si 2 down to 0.06 K. The crystals have been characterized by magnetization and specific heat measurements. We do not detect any electronic magnetic signal. Our result rules out a magnetic phase transition as the origin of the non-Fermi-liquid behavior of the specific heat and electrical resistivity observed at low temperature. ͓S0163-1829͑97͒02206-6͔The Kondo lattice compound CePt 2 Si 2 crystallizes in the CaBe 2 Ge 2 -type tetragonal structure ͑space group P4/nmm).1 Its Kondo temperature as determined by specific heat is T K Ӎ 70 K.2 At low temperature, its specific heat, electrical resistivity, and magnetic susceptibility display nonFermi-liquid behavior.2,3 Whereas the thermal behavior of the specific heat C and electrical resistivity follow the predictions for a Fermi-liquid system in the range 4-10 K, at low temperature they strongly deviate from the expected behavior. The Sommerfeld ratio C/T increases steeply as the temperature T decreases and concomitantly has an approximate linear temperature dependence.2 It has been argued that a collapse of the magnetic susceptibility in the c plane occurs below 4 K, although this conclusion has been reached after applying a large correction to the measured susceptibility.3 This correction was supposed to take into account an impurity contribution to the susceptibility. The low temperature dependence of the Sommerfeld ratio, resistivity, and susceptibility may reflect a low temperature magnetic phase transition. A more exciting possibility is that CePt 2 Si 2 is an example of a non-Fermi-liquid system. [4][5][6] If CePt 2 Si 2 has a magnetic phase transition at low temperature, this phase is certainly characterized by small magnetic moments since otherwise it would have been already detected. The most efficient method to unravel such a phase transition is to perform muon spin relaxation (SR͒ experiments.7 Here we report such experiments which show that CePt 2 Si 2 does not display any signature of static electronic magnetism. This is in contrast to most strongly correlated electron compounds for which SR experiments have detected static magnetism.
7CePt 2 Si 2 bulk materials have been prepared by direct combination of the high quality elements ͑Ce : 4N, Pt : 4 N, and Si : 6N5͒. The starting elements ͑for a total weight of nearly 10 g͒ were melted in a water-cooled copper crucible heated with a high frequency generator under a purified argon atmosphere. To improve homogeneity, the bulks were turned over and remelted several times. The weight loss is negligible using this way to prepare silicides. The material was then introduced in a triarc furnace under inert gas, equipped with a Czochralski puller.8 Two single crystals ͑the c axis was either along or perpendicular to the pulling axis͒ were grown from the same bulk starting composition using the same seed. The single crystals were checked by conventional x-ray powder diffraction and their ...