Metal–organic framework MIL-100(Fe) for artificial kidney application

Liu, Chang; Cao, Yimeng; Yan, Xiu‐Ping

doi:10.1039/c4ra05111d

Cited by 38 publications

(22 citation statements)

References 24 publications

(30 reference statements)

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“…There are also several reports suggesting nano-MIL-100 (Fe) as a safe and stable capsule for several small molecule drugs. As in Figure 1 a, benzene tricarboxylic ligands in MIL-100 have lost all of their hydrogens, and all acidic functional groups are attached to the metallic cluster [ 24 ]. Considering that the π-π interactions between aromatic rings act in the range of 3.5 Angstroms [ 25 ], and the distance between the two BTC rings in a pore of MIL-100 is about 5.763 Å, a non-covalent π-π stacking between BTC aromatic rings and aromatic rings of TC or DOX can be anticipated.…”

Section: Resultsmentioning

confidence: 99%

Application of Metal-Organic Framework Nano-MIL-100(Fe) for Sustainable Release of Doxycycline and Tetracycline

2017

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Nanostructures of MIL-100 were synthesized and used as a drug delivery platform for two members of the Tetracycline family. Doxycycline monohydrate (DOX) and Tetracycline hydrochloride (TC) were loaded separately on nano-MIL-100 (nanoparticles of drug@carrier were abbreviated as DOX@MIL-100 and TC@MIL-100). Characterizations were carried out using FT-IR, XRD, BET, DLS, and SEM. The FT-IR spectra revealed that the drugs were loaded into the framework of the carrier. The XRD patterns of DOX@MIL-100 and TC@MIL-100 indicated that no free DOX or TC were present. It could be concluded that the drugs are well dispersed into the pores of nano-MIL-100. The microporosity of the carrier was confirmed by BJH data. BET analysis showed a reduction in the free surface for both DOX@MIL-100 and TC@MIL-100. The release of TC and DOX was investigated, and it was revealed that MIL-100 mediated the drug solubility in water, which in turn resulted in a decrease in the release rate of TC (accelerating in DOX case) without lowering the total amount of released drug. After 48 h, 96 percent of the TC was sustain released, which is an unprecedented amount in comparison with other methods.

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Section: Resultsmentioning

confidence: 99%

Application of Metal-Organic Framework Nano-MIL-100(Fe) for Sustainable Release of Doxycycline and Tetracycline

2017

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“…The removal of toxin creatinine was also investigated by Fe‐MOFs. For instance, Yang et al applied MIL‐100(Fe) for the adsorptive removal of creatinine from PBS solution . The results indicated that MIL‐100(Fe) had a fast creatinine adsorption rate with the removal efficiency of 97.6% less than 2 h at a concentration of 200 mg L −1 and a adsorption capacity of 190.5 mg g −1 (nearly 7.6 times than that of carbon nanotubes).…”

Section: Applicationsmentioning

confidence: 99%

“…In consideration of the excellent adsorbability and reusability of the MIL‐100(Fe) skeleton, He et al constructed a Cu(I)‐modified MIL‐100(Fe) via a vapor‐reduction strategy and used it for the capture of benzothiophene. It was observed that the saturated capacity of Cu(I)/MIL‐100(Fe) was 0.353 mmol g −1 , much higher than pure MIL‐100(Fe) (0.139 mmol g −1 ).…”

Section: Applicationsmentioning

confidence: 99%

State‐of‐the‐Art Advances and Challenges of Iron‐Based Metal Organic Frameworks from Attractive Features, Synthesis to Multifunctional Applications

Xia

Wang

Huang

et al. 2018

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142

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The ORCID identification number(s) for the author(s) of this article can be found under https://doi.org/10.1002/smll.201803088.Metal organic frameworks (MOFs), as an original kind of organic-inorganic porous material, are constructed with metal centers and organic linkers via a coordination complexation reaction. Among uncountable MOF materials, iron-containing metal organic frameworks (Fe-MOFs) have excellent potential in practical applications owing to their many fascinating properties, such as diverse structure types, low toxicity, preferable stability, and tailored functionality. Here, recent research progresses of Fe-MOFs in attractive features, synthesis, and multifunctional applications are described. Fe-MOFs with porosity and tailored functionality are discussed according to the design of building blocks. Four types of synthetic methods including solvothermal, hydrothermal, microwave, and dry gel conversion synthesis are illustrated. Finally, the applications of Fe-MOFs in Li-ion batteries, sensors, gas storage, separation in gas and liquid phases, and catalysis are elucidated, focusing on the mechanism. The aim is to provide prospects for extending Fe-MOFs in more practical applications.Iron-Based Metal Organic Frameworks www.advancedsciencenews.com

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“…Tổng hợp MIL-100(Fe) bằng phương pháp thủy nhiệt với thành phần hỗn hợp phản ứng 1,0 FeSO4: 0,67 1,3,5-BTC: 3,0 HF: 1,2 HNO3: 280 H2O được thực hiện như sau: Hòa tan trimesic acid vào nước ở 80 o C (1); FeSO4.7H2O vào nước (2). Cho (2) vào (1) khuấy khoảng 30 phút, thêm HNO3, sau đó vừa lắc vừa cho từ từ từng giọt HF vào.…”

Section: Tổng Hợp Mil-100(fe)unclassified

A study on the synthesis of MIL-100(Fe) and its application in the catalytic degradation of methylene blue

Tran

Huynh

2018

Sci. Tech. Dev. J. - Nat. Sci.

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In the present paper, a study on the synthesis of MIL-100(Fe) by hydrothermal process and its application in the catalytic degradation of methylene blue (MB) was demonstrated. The obtained samples were characterized by X-ray Diffraction (XRD), scaning electron microscope (SEM), Fourier-transform infrared spectroscopy (FT-IR), Brunauer, Emmett and Teller (BET) and energy-dispersive X-ray spectroscopy (EDX). The results showed that the synthesized MIL- 100(Fe) exhibited high crystallinity and surface area. Its catalytic activity was evaluated by measuring the rate of conversion of MB after oxidation reaction by H2O2. The results indicated that the MIL-100(Fe) showsed high catalytic activity for the oxidation reaction of MB and at pH = 10, MB was degraded almost completely after after 3 hours of presence of the catalyst.

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Metal–organic framework MIL-100(Fe) for artificial kidney application

Cited by 38 publications

References 24 publications

Application of Metal-Organic Framework Nano-MIL-100(Fe) for Sustainable Release of Doxycycline and Tetracycline

Application of Metal-Organic Framework Nano-MIL-100(Fe) for Sustainable Release of Doxycycline and Tetracycline

State‐of‐the‐Art Advances and Challenges of Iron‐Based Metal Organic Frameworks from Attractive Features, Synthesis to Multifunctional Applications

A study on the synthesis of MIL-100(Fe) and its application in the catalytic degradation of methylene blue

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