Abstract:<b>We report, for the first time, observations of mesoscopically
homogeneous but macroscopically heterogenous water dynamics in self-assembled
materials by a new, spatially resolved infrared (IR) pump vibrational sum
frequency generation (VSFG) probe microscope. Using this new technique, we spatially
resolved dynamics of water bounded by host-guest, self-assembled sheets comprised
of sodium dodecyl sulfate (SDS) and β-cyclodextrin (β-CD). We found that the strong hydrogen-bond interactions
between β-CD
a… Show more
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