An experimental study on the tensile stress-strain curves of interlayer (layer-by-layer) unidirectional hybrid FRP composites was conducted aiming at evaluating the corresponding hybrid effect and pseudo-ductility of this innovative solution. Different combinations of the following dry unidirectional fabric materials, also varying the number of layers, were adopted in tests: high-modulus carbon, standard carbon, E-glass, and basalt. The composites were produced layer-by-layer by hand lay-up method, using an epoxy-based resin as matrix. The results have shown a strain increase at failure of both standard carbon and high-modulus carbon fibres with the volume decrease of these materials in hybrid combinations. It was also concluded that combining high-modulus carbon with E-glass, high-modulus carbon with basalt, or high-modulus carbon with standard carbon can lead to very good pseudo-ductile tensile behaviour. Finally, it should be highlighted that an existing analytical model in the literature was satisfactorily adopted to predict the tensile response of these hybrid composites.