Yttrium-stabilized
zirconia (YSZ)-based mixed potential-type NO
x
sensors have broad application prospects in
automotive exhaust gas detection. Great efforts continue to be made
in developing high-performance sensitive electrode materials for mixed
potential-type NO2 gas sensors. However, only five kinds
of new sensing electrode materials have been developed for this type
of gas sensor in the last 3 years. In this work, four different tree-based
machine learning models were trained to find potentially sensitive
electrode materials for NO2 detection. More than 400 materials
were selected from 8000 materials by the above machine learning models.
To further verify the reliability of the model, 13 of these materials
containing unexploited elements were selected as sensitive electrode
materials for making sensors and testing their gas-sensing performances.
The experimental results showed that all 13 materials exhibited good
gas-sensing performance for NO2. More interestingly, an
electrode material BPO4, which does not contain any metal
elements, was also screened out and showed good sensing properties
to NO2. In a short period of time, 13 new sensitive electrode
materials for NO2 detection were targeted and screened,
which was difficult to achieve by a trial-and-error procedure.