“…Different A&O realizations have been proposed and demonstrated, 1 , 2 , 3 , 4 such as adiabatic 5 , 6 , 7 , 8 and non‐adiabatic A&O, 9 , 10 , 11 , 12 , 13 A&O along one, 11 , 14 , 15 two, 6 or three dimensions, 16 , 17 , 18 , 19 using linearly 10 , 11 , 14 or circularly 15 polarized pulses, employing single 14 , 15 or multiple pulses, 9 , 10 , 16 , 18 utilizing optical 10 , 14 , 16 and/or terahertz (THz) 10 , 20 , 21 pulses, optical centrifuges, 6 alignment in helium droplets, 14 , 15 to name just a few developments. In addition to the various practical applications of A&O in molecular sciences, including, but not limited to rotational coherence spectroscopy (which can be used to determine accurate rotational constants 22 , 23 , 24 , 25 ), chemical reaction control, isotope and photofragment separation, and molecule trapping, the appearance of attochemistry 26 , 27 , 28 has stimulated renewed interest in A&O dynamics. Since molecular rotations typically pr...…”