Conjugated polymers doped with fullerenes show excellent photoconversion efficiencies. However, due to the poor solubility of pure C60 in common organic solvents, it was thought that some chemical modifications to C60 were required in order to load conjugated polymers with comparable weights of fullerene. Here, we report a novel way to load large amounts of unmodified C60 fullerene into the conjugated polymer poly(2‐methoxy‐5‐(2′‐ethylhexoxy)‐1,4‐phenylenevinylene), MEH‐PPV. The principle of our approach is to separate the film‐deposition stage from the material‐solidification stage. That is, materials are quickly solidified from dilute solution into colloidal particles, which are large enough to be collected by electrophoretic deposition. Deposition from a mixture of separate suspensions of MEH‐PPV and C60 fullerene resulted in films consisting of isolated particles. In contrast, by using a suspension made of a dilute solution of MEH‐PPV and C60, which was so dilute that traditional techniques such as spin‐coating were not applicable, an MEH‐PPV film doped with 20 mol‐% C60, corresponding to an almost 1:1 ratio by weight of molecularly dispersed C60, was easily obtained. To the best of our knowledge, this is the first report on the successful loading of an equivalent weight ratio of unmodified C60 molecules into MEH‐PPV.