“…Synchronous optical pumping is a well-established technique in which atomic coherence is produced by optically pumping the atoms at the rate of their Larmor precession, thus creating a resonance at nonzero magnetic field. It is implemented by modulating the light amplitude [6,7], frequency [8,9] or polarization [10][11][12]. This method has been widely used in atomic magnetometry [13,14], and also, in precision measurement of permanent electric-dipole moment [15][16][17] In synchronous optical pumping experiments, a spectrum containing multiple magnetic resonances is produced due to interaction of atoms with the frequency sidebands of modulated light [6,7].…”