h i g h l i g h t s A magnetic anisotropy of the ferromagnetic Ni nanowires was observed. The P(VDFeTrFE) glass transition has an influence on the NWs Ni/P(VDFeTrFE) 0.3% vol composite magnetic properties. The NWs Ni/P(VDFeTrFE) composite was polarized to obtain a significant piezoelectric coefficient of 7 pC N À1. The magnetoelectric coefficient reached the high value of 237 V/(m Oe).