“…[6,13,14] In this context, thin films display a great potential with respect to bulk materials for their possible integration in micro/ nanosystems for the fabrication of new-concept devices such as actuators, valves, energy harvesters, and solid-state microrefrigerators. [15,16] Nonetheless, the intimate link between magnetic and structural degrees of freedom and the peculiar hierarchical twin-within-twin martensitic structure makes epitaxial films a unique platform for the precise control of structure and magnetism from the atomic to the macroscale.Magnetic shape memory materials hold a great promise for next-generation actuation devices and systems for energy conversion, thanks to the intimate coupling between structure and magnetism in their martensitic phase. Here novel magnetic shape memory free-standing nanodisks are proposed, proving that the lack of the substrate constrains enables the exploitation of new microstructure-controlled actuation mechanisms by the combined application of different stimuli-i.e., temperature and magnetic field.…”