Magnetic exchange driven proximity effect at a magnetic-insulator-topological-insulator (MI-TI) interface provides a rich playground for novel phenomena as well as a way to realize low energy dissipation quantum devices. Here we report a dramatic enhancement of proximity exchange coupling in the MI/magnetic-TI EuS=Sb 2−x V x Te 3 hybrid heterostructure, where V doping is used to drive the TI (Sb 2 Te 3 ) magnetic. We observe an artificial antiferromagneticlike structure near the MI-TI interface, which may account for the enhanced proximity coupling. The interplay between the proximity effect and doping in a hybrid heterostructure provides insights into the engineering of magnetic ordering. The time-reversal symmetry (TRS) breaking and surface band gap opening of a topological insulator (TI) are essential ingredients necessary for towards the observation of novel quantum phases and realization for TI-based devices [1,2]. In general, there are two approaches to break the TRS: transitional-metal (TM) ion doping [3][4][5] and magnetic proximity effect where a magnetic insulator (MI) adlayer induces exchange coupling [3,[6][7][8]. Doping TM impurities into a TI will introduce a perpendicular ferromagnetic (FM) anisotropy and provide a straightforward means to open up the band gap of a TI's surface state, with profound influence to its electronic structure [4,[9][10][11][12][13][14]. In particular, quantum anomalous Hall effect (QAHE), where quantum Hall plateau and dissipationless chiral edge channels emerge at zero external magnetic field, has recently been realized in Cr-doped and V-doped TIs [9,10,[15][16][17][18][19][20]. Ideally, compared to the doping method, proximity effect has a number of advantages, including spatially uniform magnetization, better controllability of surface state, freedom from dopant-induced scattering, as well as preserving TI intrinsic crystalline structure, etc. [21,22]. However, due to the inplane anisotropy and low Curie temperature, such MIs are usually too weak to induce strong proximity magnetism in a TI. In fact, compared to a magnetically doped TI which can induce as large as a 50 meV surface band gap [4], the EuS-TI system has only a 7 meV gap opening due to the strongly localized Eu f orbitals [23]. Therefore, the enhancement of proximity magnetism is highly desirable to make it a valuable approach as doping hence takes full advantage.In this Letter, we report significant enhancement of the proximity effect in MI EuS/magnetic-TI Sb 2−x V x Te 3 hybrid heterostructure. Using polarized neutron reflectometry (PNR), we inferred an increase of proximity magnetization per unit cell (u.c.) in TI, from 1.2μ B =u:c. to 2.7μ B =u:c. at x ¼ 0.1 doping level. High-resolution transmission electron microscopy (HRTEM) identifies the TI-EuS interfacial sharpness and excludes the false positive magnetism signal from interdiffused Eu ions into a TI. Furthermore, the proximity effect enhancement is accompanied by a decrease of the interfacial magnetization of EuS, resulting in an exotic antiferro...