The magnetic properties of the hole͑x͒ doped Mott-Hubbard, antiferromagnetic insulator, NdTiO 3 , have been investigated in Nd 1−x TiO 3 . For the materials in 0.010͑6͒ Յ x Յ 0.112͑4͒, a correlation between the structural and magnetic properties is discussed with respect to the Ti-O-Ti angles and the Ti-O bond distances. For 0.010͑6͒ Յ x Յ 0.071͑10͒, long-range magnetic order is observed through low-temperature neutron diffraction and heat capacity. Néel ordering temperatures of 88.2 and 61.9 K are determined, respectively, for x = 0.019͑6͒ and x = 0.064͑10͒. From high-resolution neutron diffraction, the Pnma magnetic structure is assigned, unambiguously, as G x C y on Ti 3+ and C y 2 on Nd 3+ . The Ti 3+ ordered moment decreases gradually from 0.45͑8͒ B for x = 0.019͑6͒ to 0.31͑7͒ B for x = 0.071͑10͒, but vanishes abruptly for higher x. Antiferromagnetic short-range order exists for 0.074͑9͒ Յ x Ͻ 0.098͑10͒ as determined by neutron diffraction and the field dependence of the susceptibility. For 29͑4͒% hole doping in Nd 1−x TiO 3 , x Ն 0.098͑10͒, all magnetic ordering is destroyed.