2002
DOI: 10.1111/j.1945-5100.2002.tb00814.x
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Low‐energy helium ion irradiation‐induced amorphization and chemical changes in olivine: Insights for silicate dust evolution in the interstellar medium

Abstract: Abstract-We present the results ofirradiation experiments aimed at understanding the structural and chemical evolution ofsilicate grains in the interstellar medium. A series of'Het irradiation experiments have been performed on ultra-thin olivine, (Mg,FehSi0 4 samples having a high surface/volume (S/V) ratio, comparable to the expected S/V ratio of interstellar dust. The energies and fluences of the helium ions used in this study have been chosen to simulate the irradiation of interstellar dust grains in super… Show more

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Cited by 114 publications
(111 citation statements)
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References 44 publications
(62 reference statements)
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“…The column of gas accelerated in such shocks, which corresponds to the irradiation fluence, is of the order of 10 16 -10 18 H + /cm 2 , for 5 to 250 nm radius-grains (Jones et al 1996). In this irradiation regime nuclear interactions with the target atoms are dominant and the grains can be amorphized as shown in various simulation experiments (Demyk et al 2001;Carrez et al 2002;Jäger et al 2003a;Brucato et al 2004;Djouadi et al 2005). In addition, the grain sizes are of the same order as the implantation range of the ions, leading to the complete amorphization of the grains.…”
Section: Introductionmentioning
confidence: 91%
See 1 more Smart Citation
“…The column of gas accelerated in such shocks, which corresponds to the irradiation fluence, is of the order of 10 16 -10 18 H + /cm 2 , for 5 to 250 nm radius-grains (Jones et al 1996). In this irradiation regime nuclear interactions with the target atoms are dominant and the grains can be amorphized as shown in various simulation experiments (Demyk et al 2001;Carrez et al 2002;Jäger et al 2003a;Brucato et al 2004;Djouadi et al 2005). In addition, the grain sizes are of the same order as the implantation range of the ions, leading to the complete amorphization of the grains.…”
Section: Introductionmentioning
confidence: 91%
“…Among the processes that could account for the disappearance of the crystalline silicates in the diffuse ISM, dust amorphization induced by ion irradiation in supernovae shock waves in the warm ISM appears to be the most efficient process as demonstrated by dedicated laboratory experiments (Demyk et al 2001;Carrez et al 2002;Demyk et al 2004). During the propagation of shock waves, the interstellar gas is ionized and the gas and dust acquire relative velocities leading to dust irradiation by gas, principally protons (e.g.…”
Section: Introductionmentioning
confidence: 99%
“…However, the uncertainty on this parameter may be a factor of two and, for example, Wang et al (1999) assumed a displacement energy of E D ≈ 25 eV for similar forsterite-type materials. Experimental studies show that, under the effect of energetic ion irradiation, silicate grains become amorphous in structure (Demyk et al 2001;Carrez et al 2002) and so the displacement energy will be lower than for a crystalline structure. We therefore adopt a displacement energy of E D = 25 eV.…”
Section: Silicate Core Sputteringmentioning
confidence: 99%
“…Further, we require a quantity for how many displacements per lattice atom (dpa) are required to observe amorphization. We set this number to be 2.5 based on the mineral irradiation experiments for enstatite (Jäger et al 2003), forsterite (Bringa et al 2007) and olivine (Demyk et al 2001;Carrez et al 2002). However, this quantity remains inaccurate as most of the above cited studies determined doses for He-irradiation to fully amorphize the minerals varying within an order of magnitude.…”
Section: Calculation Of Dust Amorphizationmentioning
confidence: 99%
“…The destructive impact of high-energy irradiation on crystalline structures by ions has been demonstrated in laboratory measurements by, e.g., Jäger et al (2003), Bringa et al (2007), Demyk et al (2001), Carrez et al (2002), mainly for low energetic cosmic rays (E > ∼ 50 keV) but rarely also for lower energies typical of stellar winds.…”
Section: Introductionmentioning
confidence: 99%