2022
DOI: 10.5194/acp-2022-313
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Long-Term Monitoring of Cloud Water Chemistry at Whiteface Mountain: The Emergence of a New Chemical Regime

Abstract: Abstract. Atmospheric aqueous chemistry can have profound effects on our environment. The importance of chemistry within the atmospheric aqueous phase was first realized in the 1970s as there was growing concern over the negative impacts on ecosystem health from acid deposition. Research at mountaintop observatories including Whiteface Mountain (WFM) showed that gas phase sulfur dioxide emissions react in cloud droplets to form sulfuric acid, which also impacted aerosol mass loadings. Cloud chemistry research … Show more

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Cited by 2 publications
(1 citation statement)
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“…Particulate sulfur is also becoming increasingly recognized as organic (Riva et al, 2019;Moch et al, 2018). At the same time sulfate and nitrate in cloud water have been decreasing at a mountaintop site in the Northeast U.S., total organic carbon in cloud water may be increasing (Lawrence et al, 2022)…”
Section: Discussionmentioning
confidence: 99%
“…Particulate sulfur is also becoming increasingly recognized as organic (Riva et al, 2019;Moch et al, 2018). At the same time sulfate and nitrate in cloud water have been decreasing at a mountaintop site in the Northeast U.S., total organic carbon in cloud water may be increasing (Lawrence et al, 2022)…”
Section: Discussionmentioning
confidence: 99%