Abstract:CuCrO2 nanocrystals were synthesized and fabricated into mesoporous thin films to study their electrochemical properties, where a strong [Li+] dependence was observed. An anodic shift in the Cu2+/+ redox potential was observed with increased [Li+] in the electrolyte, in addition to the growth of a new redox feature at E1/2=−0.43 V vs Fc+/0. This new feature was attributed to Cu2+/+ redox chemistry accompanied by Li+ occupation in copper vacancy surface defects. The equilibrium constant and maximum charge for L… Show more
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