Linkage‐Mediated Electronic Structure Modulation in Multicomponent Covalent Organic Frameworks for Dramatically Promoted Photocatalytic Hydrogen Evolution
Yu Yan,
Yanming Zhao,
Xikai Chen
et al.
Abstract:Linkage chemistry is an essential aspect to covalent organic framework (COF) applications; it is highly desirable to precisely modulate electronic structure mediated directly by linkage for efficient COF‐based photocatalytic hydrogen evolution, which however, remains substantially challenging. Herein, as a proof of concept, a collection of robust multicomponent pyrene‐based COFs with abundant donor‐acceptor (D‐A) interactions has been judiciously designed and synthesized through molecularly engineering linkage… Show more
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