Abstract:We propose the design of 1D photonic crystals and microcavities in which fluorine-indium codoped cadmium oxide (FICO) nanocrystal based layers and layers of diarylethene-based polyester (pDTE) are alternated or embedded in a microcavity. The irradiation with UV light results in two different behaviours: i) it dopes the FICO nanocrystals inducing a blue shift of their plasmonic resonances; ii) it changes the real part of the refractive index of the photochromic pDTE polymer. These two behaviours are combined in… Show more
“…These structures consist of dielectric lattices made of thin film with different refractive indexes, alternated periodically, that interact with light generating specific frequency regions forbidden photon propagation, namely photonic band gaps (PBGs). Microcavities and DBRs were demonstrated for several applications including photon recycling in photovoltaics [36], sensing [35,[37][38][39][40][41][42] and optical switchers [43][44][45]. With regards to emission control, these planar lattices are of interest thanks to the spectral and directional redistribution of the photoluminescence oscillator strength [46], as already demonstrated for polymers and organic dyes [47][48][49][50][51][52][53][54][55] as well as inorganic emitters [54,56].…”
Thanks to solution processability and broad emission in the visible spectral range, 2D hybrid perovskite-like materials are interesting for the realization of large area and flexible lighting devices. However, the deposition of these materials requires broad-spectrum solvents that can easily dissolve most of the commercial polymers and make perovskites incompatible with flexible photonics. Here, we demonstrated the integration of broadband-emitting (EDBE)PbCl4 (where EDBE = 2,2-(ethylenedioxy)bis(ethylammonium)) thin films with a solution-processed polymer planar microcavities, employing a sacrificial polymer multilayer. This approach allowed for spectral and angular redistribution of the perovskite-like material, photoluminescence, that can pave the way to all-solution-processed and flexible lightning devices that do not require complex and costly fabrication techniques.
“…These structures consist of dielectric lattices made of thin film with different refractive indexes, alternated periodically, that interact with light generating specific frequency regions forbidden photon propagation, namely photonic band gaps (PBGs). Microcavities and DBRs were demonstrated for several applications including photon recycling in photovoltaics [36], sensing [35,[37][38][39][40][41][42] and optical switchers [43][44][45]. With regards to emission control, these planar lattices are of interest thanks to the spectral and directional redistribution of the photoluminescence oscillator strength [46], as already demonstrated for polymers and organic dyes [47][48][49][50][51][52][53][54][55] as well as inorganic emitters [54,56].…”
Thanks to solution processability and broad emission in the visible spectral range, 2D hybrid perovskite-like materials are interesting for the realization of large area and flexible lighting devices. However, the deposition of these materials requires broad-spectrum solvents that can easily dissolve most of the commercial polymers and make perovskites incompatible with flexible photonics. Here, we demonstrated the integration of broadband-emitting (EDBE)PbCl4 (where EDBE = 2,2-(ethylenedioxy)bis(ethylammonium)) thin films with a solution-processed polymer planar microcavities, employing a sacrificial polymer multilayer. This approach allowed for spectral and angular redistribution of the perovskite-like material, photoluminescence, that can pave the way to all-solution-processed and flexible lightning devices that do not require complex and costly fabrication techniques.
“…In photonic crystals, the periodic modulation of the refractive index in one, two or three dimensions gives rise to energy regions in which light is not transmitted through the crystal. The integration of materials with switchable optical properties in the infrared, such as photochromic polymers (Toccafondi et al, 2014) and infrared plasmonic nanomaterials (Guo et al, 2016;Kriegel et al, 2016), in one-dimensional photonic crystals has been proposed previously (Kriegel and Scotognella, 2018). Furthermore, the deposition of a VO 2 layer onto a onedimensional photonic crystal has been theoretically studied by Rashidi et al (2018) and experimentally studied by Singh et al (Singh et al(2020).…”
The optical properties of vanadium dioxide (VO2) can be tuned via metal-insulator transition. In this work, different types of one-dimensional photonic structure-based microcavities that embed vanadium dioxide have been studied in the spectral range between 900 nm and 2000 nm. In particular, VO2 has been sandwiched between: i) two photonic crystals made of SiO2 and ZrO2; ii) two aperiodic structures made of SiO2 and ZrO2 that follow the Thue-Morse sequence; iii) two disordered photonic structures, made of SiO2 and ZrO2 in which the disorder is introduced either by a random sequence of the two materials or by a random variation of the thicknesses of the layers; iv) two four material-based photonic crystals made of SiO2, Al2O3, Y2O3, and ZrO2. The ordered structures i and iv show, respectively, one and two intense transmission valleys with defect modes, while the aperiodic and disordered structures ii and iii show a manifold of transmission valleys due to their complex layered configurations. The metal-insulator transition of VO2, controlled by temperature, results in a modulation of the optical properties of the microcavities.
“…[5][6][7] There exist numerous reports in which optical features of various kinds of these structures have been investigated. [8][9][10][11][12][13] They have been widely proposed in fabrications of not only light sources such as lasers/diodes [14,15] but also detectors and transducers, [15] all optical filters, mirrors, and switches. [16][17][18][19][20][21][22][23][24][25][26] Nevertheless, these structures are still on tops of attention for new photonic elements design due to their unique characteristics.…”
Optical features of a semiconductor–dielectric photonic crystal are studied theoretically. Alternating layers of micrometer sized SiO2/InSb slabs are considered as building blocks of the proposed ideal crystal. By inserting additional layers and disrupting the regularity, two more defective crystals are also proposed. Photonic band structure of the ideal crystal and its dependence on the structural parameters are explored at the first step. Transmittance of the defective crystals and its changes with the thicknesses of the layers are studied. After extracting the optimum values for the thicknesses of the unit cells of the crystals, the optical response of the proposed structures at different temperatures and incident angles are investigated. Changes of the defect layers’ induced mode(s) are discussed by taking into consideration of the temperature dependence of the InSb layer permittivity. The results clearly reflect the high potential of the proposed crystals to be used at high temperature terahertz technology as a promising alternative to their electronic counterparts.
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