Liberating Lithium Ions from Polymer Matrix via Harnessing Ion‐Dipole Interaction Toward Stable Solid‐State Lithium Metal Batteries
Dashan Zhang,
Zicheng Luo,
Hongfei Xu
et al.
Abstract:Although polymer electrolytes have shown great potential in solid‐state lithium metal batteries (LMBs), the polymer chain segments anchor the movement of lithium ions (Li+), which induces the low ionic conductivity of the electrolytes and limits their application. Herein, a strategy of harnessing ion‐dipole interactions is proposed to liberate lithium ions from polymer chains. The adiponitrile (ADN) molecular dipole with strong bond dipole moment (C≡N, 11.8 × 10−30 C m) is introduced into the polyvinylidene f… Show more
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