Lewis Säure‐Getriebene Inverse Hydrid‐Shuttle Katalyse
Benjamin T. Jones,
Nuno Maulide
Abstract:Inverse hydride shuttle catalysis provides a multicomponent platform for the highly efficient synthesis of alkaloid frameworks with exquisite diastereoselectivity. However, a number of limitations hinder this method, primarily the strict requirement for highly electron‐deficient acceptors. Herein, we present a general Lewis Acid‐driven approach to address this constraint, and have developed two broad strategies enabling the modular synthesis of complex azabicycles that were entirely unattainable using the prev… Show more
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