1997
DOI: 10.1364/ao.36.007718
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Lasing in active, sub-mean-free path-sized systems with dense, random, weak scatterers

Abstract: We report enhanced emission and gain narrowing in Rhodamine 590 perchlorate dye in an aqueous suspension of polystyrene microspheres. A systematic experimental study of the threshold condition for and the gain narrowing of the stimulated emission over a wide range of dye concentrations and scatterer number densities showed several interesting features, even though the transport mean free path far exceeded the system size. The conventional diffusive-reactive approximation to radiative transfer in an inhomogeneo… Show more

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Cited by 39 publications
(24 citation statements)
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“…The latter is recieving much attention in recent years in the context of random lasers [13][14][15]. To fix ideas, consider the case of a single mode optical fibre doped with Er 3+ , say, optically pumped and intentionally disordered refractively.…”
mentioning
confidence: 99%
“…The latter is recieving much attention in recent years in the context of random lasers [13][14][15]. To fix ideas, consider the case of a single mode optical fibre doped with Er 3+ , say, optically pumped and intentionally disordered refractively.…”
mentioning
confidence: 99%
“…The lasing threshold could be reduced by more than two orders of magnitude as compared to pure dye, when the density of scatterers ranged from 5 ¢ 10 9 /cc to 2 5 ¢ 10 12 /cc. In one particular study, a thousand-fold increase in the peak emission intensity was observed upon addition of scatterers [19]. For a range of dye and scatterer concentrations, bi-modal emission, with competition between the modes was seen.…”
mentioning
confidence: 88%
“…Coherent laser emission from such a random amplifying medium has been reported, and has become a subject of active research [2][3][4][5][6][7][8][9][10][11][12][13][14][15][16][17][18][19][20]. Recently, we had initiated a theoretical study [2] of light-wave propagation in a one-dimensional coherently amplifying medium where amplification is introduced phenomenologically by adding a negative imaginary part to the otherwise real dielectric constant, assumed spatially random.…”
Section: Introductionmentioning
confidence: 99%
“…We think this is essentially the result of the interplay of localization and coherent amplification in the presence of nonlinearity, i.e., the light-intensity dependence of 0 that has been neglected in the present linear analysis. Finally, we would like to report briefly on a rather curious result obtained in a recent experiment [20] where we have investigated experimentally the random laser action in a dilute aqueous suspension of polystyrene microspheres containing the pumped laser dye rhodamine 590. The low refractive index contrast of the water/polystyrene system and the low concentration of scatterers gave an estimated meanfree path much greater than the sample size.…”
Section: Introductionmentioning
confidence: 99%