2018
DOI: 10.1038/s41467-018-04395-2
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Large quantum-spin-Hall gap in single-layer 1T′ WSe2

Abstract: Two-dimensional (2D) topological insulators (TIs) are promising platforms for low-dissipation spintronic devices based on the quantum-spin-Hall (QSH) effect, but experimental realization of such systems with a large band gap suitable for room-temperature applications has proven difficult. Here, we report the successful growth on bilayer graphene of a quasi-freestanding WSe2 single layer with the 1T′ structure that does not exist in the bulk form of WSe2. Using angle-resolved photoemission spectroscopy (ARPES) … Show more

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Cited by 140 publications
(134 citation statements)
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“…16 Furthermore, monolayer WTe 2 is the only member of this materials class that is known to realize the topologically nontrivial 1T structure as its stable ground state. 16,24,25,46 The crystal structure is generated from the tetragonal 1T configuration by a lattice distortion: 16,44,45 the original 1T configuration is composed of three hexagonal layers in rhombohedral ABC stacking with one W layer sandwiched between two Te layers. A structural distortion then shifts the W atoms along the b direction to form zigzag chains.…”
Section: Introductionmentioning
confidence: 99%
“…16 Furthermore, monolayer WTe 2 is the only member of this materials class that is known to realize the topologically nontrivial 1T structure as its stable ground state. 16,24,25,46 The crystal structure is generated from the tetragonal 1T configuration by a lattice distortion: 16,44,45 the original 1T configuration is composed of three hexagonal layers in rhombohedral ABC stacking with one W layer sandwiched between two Te layers. A structural distortion then shifts the W atoms along the b direction to form zigzag chains.…”
Section: Introductionmentioning
confidence: 99%
“…Experimental relevance and summary.-Now we briefly discuss the experimental relevance for our proposal. QSHIs with large inverted gaps [44][45][46][47][48][49][50][51][52][53][54][55][71][72][73] in proximity to cuprate or iron-based superconductors [38][39][40][57][58][59][60][61] could provide promising platforms to detect our predictions. For concreteness, we take the inverted InAs/GaSb bilayer and WTe 2 monolayer to estimate µ c x(y) .…”
Section: Arxiv:190509308v1 [Cond-matsupr-con] 22 May 2019mentioning
confidence: 99%
“…This condition indeed corresponds to the QSHI phase with a large inverted gap or equivalently an indirect bulk gap. It is likely realized in the inverted InAs/GaSb bilayer [71][72][73], WTe 2 monolayer [44][45][46][47][48], functionalized MXene [49,50], Bismuthene on SiC [51,52], PbS monolayer [53][54][55], etc. To test the analytical results, we discretize the model (1), put it on a lattice, choose a proper set of parameters (satisfying inequality (8)) and calculate the energy spectrum in a ribbon geometry.…”
Section: Arxiv:190509308v1 [Cond-matsupr-con] 22 May 2019mentioning
confidence: 99%
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“…Specifically, the propagation direction of the carriers of the same spin is reversed at the opposite edge. Such unique transport properties enable QSH systems to own promising applications in low-power electronics and spintronics [9][10][11][12] . In the early years, the studies of QSH systems mainly focus on group-VI monolayers (e.g., graphene 1,2 and silicene 13,14 ) and semiconductor quantum wells (e.g., HgTe/CdTe 3,4 and InAs/GaSb 15,16 ).…”
Section: Introductionmentioning
confidence: 99%