“…Much effort has been made to improve the wettability of the substrate and suppress the coffee ring effect, [44,45] such as solvent engineering for balancing the Marangoni flow and capillary flow [46,47] and interface engineering for adjusting the surface energy. [34,48] However, the EQE of inkjet-printed PeLEDs is still limited to 9.6% with red emission and 13.9% with green emission, [33,49] and the device area is limited to 16 cm 2 [50] ; both still lag behind that of spin-coated or blade-coated PeLEDs on rigid substrates. [21,30] In this work, we demonstrate efficient, flexible, and large-area PeLEDs using inkjet printing.…”