The development of
high-performance self-powered sensors
in advanced
composites addresses the increasing demands of various fields such
as aerospace, wearable electronics, healthcare devices, and the Internet-of-Things.
Among different energy sources, the thermoelectric (TE) effect which
converts ambient temperature gradients to electric energy is of particular
interest. However, challenges remain on how to increase the power
output as well as how to harvest thermal energy at the out-of-plane
direction in high-performance fiber-reinforced composite laminates,
greatly limiting the pace of advance in this evolving field. Herein,
we utilize a temperature-induced self-folding process together with
continuous carbon nanotube veils to overcome these two challenges
simultaneously, achieving a high TE output (21 mV and 812 nW at a
temperature difference of 17 °C only) in structural composites
with the capability to harvest the thermal energy from out-of-plane
direction. Real-time self-powered deformation and damage sensing is
achieved in fabricated composite laminates based on a thermal gradient
of 17 °C only, without the need of any external power supply,
opening up new areas of autonomous self-powered sensing in high-performance
applications based on TE materials.