In
developing countries, waterborne diseases caused by the pathogenic
bacteria are afflicting people who lack access to clean drinking water
and live in poor sanitary conditions. User-friendly and low-cost point-of-use
(POU) disinfection systems have become the key solution for providing
safe drinking water. Herein, a biomass-based renewable film filter
with good mechanical strength, porous network structure, and robustly
immobilized silver nanoparticles was facilely fabricated via Fe(III) cross-linking-induced collagen fibers (CFs) and gallic acid-protected
silver nanoparticle (GA@AgNP) self-assembly. Scanning electron microscopy,
X-ray photoelectron spectroscopy, thermogravimetric analysis, and
X-ray diffraction were employed to characterize the GA@AgNPs–Fe-CF
composite film. This film exhibited both excellent bacterial anti-adhesive
and bactericidal activities, which effectively prevented biofouling
during the filtration process because of the anionic GA@AgNPs. As
the bactericidal filter is driven by gravity, 1 L of the natural water
sample was treated by the GA@AgNPs–Fe-CF film for 20 min, and
the water quality was in full compliance with the drinking water guidelines
of the World Health Organization (WHO), demonstrating the potential
application of the proposed filter in POU water disinfection.