[1] We report Hf isotope compositions of 79 lavas that record the early ($5-95 Ma) history of the Galápagos plume volcanism. These include lavas from the Caribbean Large Igneous Province (CLIP; $95-70 Ma), the accreted Galápagos paleo-hot spot track terranes (54-65 Ma) of Costa Rica (Quepos, Osa and Burica igneous complexes), and the Galápagos hot spot tracks (<20 Ma) located on the Pacific seafloor (Cocos, Carnegie, Malpelo, and Coiba Ridges and associated seamounts). These samples have previously been well characterized in terms of major and trace elements, Sr-Nd-Pb isotopes and Ar/Ar ages. As a result of the relative immobility of the high field strength and rare earth elements during synand post-emplacement hydrothermal activity and low-temperature alteration, combined Lu-Hf and Sm-Nd isotope systematics, when used in conjunction with Pb isotopes, provide a particular powerful tool, for evaluating the source compositions of ancient and submarine lavas. The combined Nd-Hf isotope data suggest that three of the isotopically distinct source components found today in the Galápagos Islands (the Floreana-like southern component, the Fernandina-like central component, and the depleted Genovesa-like eastern component) were present in the CLIP already by 95-70 Ma. The fourth Pinta-like northern component is first recorded at about 83-85 Ma by volcanism taking place during the transition from the plume head/CLIP to plume tail stage and has then been present in the hot spot track continuously thereafter. The identification of the unique northern and southern Galápagos Plume Hf-Nd-Pb isotope Pb and lower DeHf, a signature typical of the northern Galápagos island Pinta.