“…They have been used extensively in studies of environmental hydrology [Friedman et al, 1964;Clark and Fritz, 1997], paleoclimatology [Johnsen et al, 1972;Merlivat and Jouzel, 1979;Jouzel et al, 1982Jouzel et al, , 1987, and cloud physics [Jouzel, 1986] Since the stable isotope composition of atmospheric moisture is intimately related to its origin, cloud fractionation, and subsequent removal from the atmosphere [•at and Matsui, 1991], the isotope ratios of atmospheric water vapor provide critical information about the mechanisms of evaporation at the surface of the Earth and of subsequent transport and phase changes in the atmosphere. Profiles of deuterium isotope ratio in atmospheric water vapor in the troposphere were measured by Ehhalt [1974], Taylor [1972Taylor [ , 1984.…”