In the case of insufficient quantitative data, qualitative evaluation information is very important for investment decision-making. However, if it is completely based on qualitative evaluation information, the results may be subjective. In response to this problem, this paper proposes a method, namely, probabilistic hesitant fuzzy cross-efficiency evaluation (PHFCEE) method, based on probabilistic hesitant fuzzy theory, cross-efficiency data envelopment analysis (CEDEA). This method uses probabilistic hesitant fuzzy sets to collect qualitative evaluation information and then uses the cross-efficiency DEA model to fuse quantitative data and qualitative information. And finally, an investment portfolio is built based on the cross-efficiency value and its variance. In addition, this article gives the specific operating steps of the PHFCEE method and uses the construction of a portfolio of 10 stocks in the China CSI 300 Index as an example to illustrate the effectiveness of this method.