Abstract:The dependence of the shape of the glow curve of LiF:Mg,Ti (TLD-100) on ionisation density was investigated using irradiation with (90)Sr/(90)Y beta rays, 60 and 250 kVp X rays, various heavy-charged particles and 0.2 and 14 MeV neutrons. Special attention is focused on the properties of high-temperature thermoluminescence; specifically, the behaviour of the high-temperature ratio (HTR) of Peaks 7 and 8 as a function of batch and annealing protocol. The correlation of Peaks 7 and 8 with average linear-energy-t… Show more
“…As shown in figure 3, the values of T max remain very nearly constant as a function of dose except for a slight increase in the temperature of maximum intensity of the HTTL. This, in fact, is observed in experimental measurements of the HTTL due to the greater relative intensity of peaks 8-10 at high dose level [40,41]. The reader should also note the increase in the concentration density of the CC at the temperatures corresponding to the thermal depletion of the TCs.…”
Section: Resultsmentioning
confidence: 78%
“…However, it deserves mention that the linear region of dose response observed for the HTTL at low dose levels extends over at most 1-2 decades of dose, whereas for peak 5, the dose response is linear over at least 5 decades of dose. In our recent studies [41] the dose response of peak 7 dose not deviate from linearity by more than ±20% (1 SD) over the dose range 10-200 mGy. However, if the dose response data for peaks 7 and 8 is fitted with a function of the form (top) and 1 • C s −1 (bottom).…”
TL kinetic theory based on delocalized recombination mechanisms is successful in predicting many characteristics of TL mechanisms when these are considered singly. However, the greater challenge of predicting a set of measured TL characteristics while using the same, or very nearly the same, parameter values has yet to be adequately addressed. In this work we apply delocalized kinetic modelling to describe four experimentally measured characteristics of the TL behaviour of peak 5 in LiF : Mg,Ti (TLD-100). These include: (i) optical absorption linear/exponentially saturating dose response of the appropriate OA bands with the experimentally measured dose filling constants; (ii) linear/supralinear TL dose response with f(D)max = 4–6 at a dose level of ∼400–600 Gy; (iii) constancy of Tmax with dose; (iv) agreement with the experimentally measured behaviour of Tmax and f(D)max with heating rate. We are successful in describing most of the details of these characteristics; however, we have failed to find parameter values which also correctly describe the dose response behaviour at low dose levels (preceding the linear, then the supralinear region) and the behaviour of f(D)max with heating rate. It is suggested that kinetic modelling based on a mixture of localized and delocalized recombination could successfully describe all the characteristics involved.
“…As shown in figure 3, the values of T max remain very nearly constant as a function of dose except for a slight increase in the temperature of maximum intensity of the HTTL. This, in fact, is observed in experimental measurements of the HTTL due to the greater relative intensity of peaks 8-10 at high dose level [40,41]. The reader should also note the increase in the concentration density of the CC at the temperatures corresponding to the thermal depletion of the TCs.…”
Section: Resultsmentioning
confidence: 78%
“…However, it deserves mention that the linear region of dose response observed for the HTTL at low dose levels extends over at most 1-2 decades of dose, whereas for peak 5, the dose response is linear over at least 5 decades of dose. In our recent studies [41] the dose response of peak 7 dose not deviate from linearity by more than ±20% (1 SD) over the dose range 10-200 mGy. However, if the dose response data for peaks 7 and 8 is fitted with a function of the form (top) and 1 • C s −1 (bottom).…”
TL kinetic theory based on delocalized recombination mechanisms is successful in predicting many characteristics of TL mechanisms when these are considered singly. However, the greater challenge of predicting a set of measured TL characteristics while using the same, or very nearly the same, parameter values has yet to be adequately addressed. In this work we apply delocalized kinetic modelling to describe four experimentally measured characteristics of the TL behaviour of peak 5 in LiF : Mg,Ti (TLD-100). These include: (i) optical absorption linear/exponentially saturating dose response of the appropriate OA bands with the experimentally measured dose filling constants; (ii) linear/supralinear TL dose response with f(D)max = 4–6 at a dose level of ∼400–600 Gy; (iii) constancy of Tmax with dose; (iv) agreement with the experimentally measured behaviour of Tmax and f(D)max with heating rate. We are successful in describing most of the details of these characteristics; however, we have failed to find parameter values which also correctly describe the dose response behaviour at low dose levels (preceding the linear, then the supralinear region) and the behaviour of f(D)max with heating rate. It is suggested that kinetic modelling based on a mixture of localized and delocalized recombination could successfully describe all the characteristics involved.
“…It has been in use essentially without modification since its initial construction and continues to be used frequently even today. In addition to cell cultures (16), the facility has been used to irradiate spores, thin layers of DNA in solution (17), 3D artificial tissue (18), TLDs (19), track etch dosimeters, and microchips. One result of irradiations using this facility was the measurement of oncogenic cell transformation as a function of LET (20, 21).…”
The Radiological Research Accelerator Facility (RARAF) is in its 50th year of operation. It was commissioned on April 1, 1967 as a collaboration between the Radiological Research Laboratory (RRL) of Columbia University, and members of the Medical Research Center of Brookhaven National Laboratory (BNL). It was initially funded as a user facility for radiobiology and radiological physics, concentrating on monoenergetic neutrons. Facilities for irradiation with MeV light charged particles were developed in the mid-1970s. In 1980 the facility was relocated to the Nevis Laboratories of Columbia University. RARAF now has seven beam lines, each having a dedicated irradiation facility: monoenergetic neutrons, charged particle track segments, two charged particle microbeams (one electrostatically focused to <1 μm, one magnetically focused), a 4.5 keV soft X-ray microbeam, a neutron microbeam, and a facility that produces a neutron spectrum similar to that of the atomic bomb dropped at Hiroshima. Biology facilities are available on site within close proximity to the irradiation facilities, making the RARAF very user friendly.
“…The separate measurement of the beta and neutron dose components in both mixed neutron-beta and mixed gamma-neutron radiation fields remains a difficult issue [1][2][3]. The applied techniques usually employ two types of dosemeters in which the efficiency of the high ionization density (HID) radiation (heavy charged particles and neutrons) relative to that of the gammas and electrons of low ionization density (LID) is different [4][5][6][7][8][9][10][11]. In this work the LID irradiations were carried out with a 90 Sr/ 90 Y beta source (mean energy ~ 0.55 MeV) but the results are equally applicable to gamma radiation of the same range of energies.…”
The results reported herein were motivated by the potential application of combined optically stimulated (OSL) and thermoluminescence (TL) measurements for separation between the beta and neutron dose components in mixed neutron-beta radiation fields. The advantages of OSL/TL are two-fold: (i) The OSL and TL readout can be carried out on the same sample and (ii) the greater efficiency of OSL to high ionization density (HID) radiation due to the excitation of F2 and F3
+ centers. The beta calibration coefficients for LiF:Mg,Ti (TLD-700) were measured using a 90Sr/90Y source calibrated at the Soreq Nuclear Research Center nuclear facility. The estimation of the neutron calibration coefficients was carried out by irradiation with broad beam fast neutrons of median energy 5 MeV and a quasi-monoenergetic neutron field of mean energy 14.8 MeV at the Physikalisch Technische Bundenanstalt. The preferential excitation of OSL following HID irradiation has been demonstrated.
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