“…In conclusion, we demonstrate a novel method for generation of structured single-cycle THz wavepackets from engineered NLMS. Such NLMS can replace conventional nonlinear crystals in THz generation systems to provide new functionalities without sacrificing efficiency, avoid phononic interactions or phase mismatch considerations, and potentially obtain larger THz bandwidths 25,26 . This unprecedented capability, which overcomes several limitations of conventional THz generation and manipulation schemes, opens the door for advanced THz technologies, such as beam multiplexing, structured-light THz imaging, single-shot spectroscopy, THz holography, particle manipulation, and structured THz light–matter interactions.…”