“…Therefore, self-frequency doubling (SFD) laser crystals, which possess laser and nonlinear optical functions simultaneously, have attracted researchers' interests. Over the past few decades, a lot of progress has been made in search for SFD laser crystals, such as Re:LiNbO 3 (Re¼ Nd, Tm, Ho) [5], Re:YAl(BO 3 ) 4 (Re¼ Nd, Yb, Er, Dy) [6], Nd: Ca 4 GdO(BO 3 ) 3 [7], Nd:GdAl 3 (BO 3 ) 4 [8] and Nd:La 2 CaB 10 O 9 [9,10]. However, the applications of these SFD laser crystals are not commercialized effectively.…”