Interfacial Electrochemistry of Catalyst-Coordinated Graphene Nanoribbons
Erik Askins,
Pouyan Navabi,
Khagesh Kumar
et al.
Abstract:The immobilization of molecular electrocatalysts on conductive electrodes is an appealing strategy for enhancing their overall activity relative to analogous molecular compounds. In this study we report on the interfacial electrochemistry of self-assembled 2D nanosheets of graphene nanoribbons (GNR-2DNS) and analogs containing a Rh-based hydrogen evolution reaction (HER) catalyst (RhGNR-2DNS) immobilized on conductive electrodes. Proton-coupled electron transfer (PCET) taking place at N-centers of the nanoribb… Show more
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