“…Inter-annual fluctuations over the past decade or so are driven by the five main driving mechanisms: (1) impact of better regulation and anti-pollution measures (EPA, 2010(EPA, , 2012Oltmans et al, 2013), (2) meteorological fluctuations (Thompson et al, 2001;Camalier et al, 2007;Zheng et al, 2007;Davis et al, 2011), (3) socio-economic changes (e.g., recession; Friedlingstein et al, 2010;Granados et al, 2012;Castellanos and Folkert Boersma, 2012), (4) increase of background levels due to intercontinental transport (Cooper, , 2012, and (5) inter-annual variability of stratospherictropospheric exchanges Lin et al, 2012a, b). Following Cooper et al (2010Cooper et al ( , 2012 and Vautard et al (2006), a general trend analysis is computed by using the percentiles to take into account the changes of the full distribution through time.…”