2014
DOI: 10.1002/ange.201310957
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Innenrücktitelbild: Cobalt Imidazolate Metal–Organic Frameworks Photosplit CO2 under Mild Reaction Conditions (Angew. Chem. 4/2014)

Abstract: Ein künstliches Photosynthesesystem wird von X. Wang und Mitarbeitern in der Zuschrift auf vorgestellt. Die Porosität eines zeolithischen Cobaltimidazolat‐Gerüsts ermöglicht das Einfangen von CO2, auf das die Liganden und Metallzentren katalytisch einwirken können. Dieses Metall‐organische Gerüst konnte in Kombination mit einem Ruthenium‐Photosensibilisator CO2 zu CO reduzieren. Unter milden Reaktionsbedingungen wurden binnen 2.5 h Umsatzzahlen von 450 erreicht.

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“…Besides the most regular approach, the authors reported an in situ growth approach to fabricate MOF-coated PNC hybrid structures, which widely enhanced the performance of the photocatalyst in CO 2 reduction . Some previous works reported a CsPbBr 3 @ZIF (zeolitic imidazolate framework) hybrid structure as a photocatalyst, where more cobalt-containing ZIFs, like ZIF-9 and ZIF-67, exhibited effective cocatalysts to advance the CO 2 activation and conversion. For conceptual proof, different CsPbBr 3 @ZIF hybrids, like CsPbBr 3 @ZIF-8 and CsPbBr 3 @ZIF-67, were included. Therefore, the research group noticed an electron consumption rate of 15.498 and 29.630 μmol g –1 h –1 for CsPbBr 3 @ZIF-8 and CsPbBr 3 @ZIF-67 individually.…”
Section: Cspbx3 Perovskites For Photocatalytic Organic Synthesis and ...mentioning
confidence: 99%
“…Besides the most regular approach, the authors reported an in situ growth approach to fabricate MOF-coated PNC hybrid structures, which widely enhanced the performance of the photocatalyst in CO 2 reduction . Some previous works reported a CsPbBr 3 @ZIF (zeolitic imidazolate framework) hybrid structure as a photocatalyst, where more cobalt-containing ZIFs, like ZIF-9 and ZIF-67, exhibited effective cocatalysts to advance the CO 2 activation and conversion. For conceptual proof, different CsPbBr 3 @ZIF hybrids, like CsPbBr 3 @ZIF-8 and CsPbBr 3 @ZIF-67, were included. Therefore, the research group noticed an electron consumption rate of 15.498 and 29.630 μmol g –1 h –1 for CsPbBr 3 @ZIF-8 and CsPbBr 3 @ZIF-67 individually.…”
Section: Cspbx3 Perovskites For Photocatalytic Organic Synthesis and ...mentioning
confidence: 99%