“…In high‐power laser system, optical isolator based on the nonreciprocal Faraday effect is a no‐negligible passive component as it can effectively isolate the deleterious backlight, which is conducive to reducing the damage to the laser source and ensuring the stability of the systems 1–6 . In pace with the development of magneto‐optical isolators toward high power, miniaturization, and low cost, 7–10 more stringent requirements are being placed on the properties of magneto‐optical materials, mainly including high Verdet constant, large size, good optical quality, high thermal conductivity, outstanding laser damage threshold, and so on 11–17 . At present, terbium gallium garnet (Tb 3 Ga 5 O 12 , TGG) single crystals are the mainstream magneto‐optical material used in the visible and near‐infrared bands, 18–20 whereas terbium aluminum garnet (Tb 3 Al 5 O 12 , TAG) has a same garnet structure with TGG 21–23 .…”