Abstract. Anthropogenic aerosols (AAs) induce global and regional
tropospheric circulation adjustments due to the radiative energy
perturbations. The overall cooling effects of AA, which mask a portion of
global warming, have been the subject of many studies but still have large
uncertainty. The interhemispheric contrast in AA forcing has also been
demonstrated to induce a major shift in atmospheric circulation. However,
the zonal redistribution of AA emissions since start of the 20th century, with a
notable decline in the Western Hemisphere (North America and Europe) and a
continuous increase in the Eastern Hemisphere (South Asia and East Asia),
has received less attention. Here we utilize four sets of single-model initial-condition large-ensemble
simulations with various combinations of external forcings to quantify the
radiative and circulation responses due to the spatial redistribution of AA
forcing during 1980–2020. In particular, we focus on the distinct climate
responses due to fossil-fuel-related (FF) aerosols emitted from the Western Hemisphere (WH) versus the Eastern Hemisphere (EH). The zonal (west to east) redistribution of FF aerosol emission since the
1980s leads to a weakening negative radiative forcing over the WH
mid-to-high latitudes and an enhancing negative radiative forcing over the
EH at lower latitudes. Overall, the FF aerosol leads to a northward shift of the Hadley cell and an equatorward shift of the Northern Hemisphere (NH) jet stream. Here, two sets of regional FF simulations (Fix_EastFF1920
and Fix_WestFF1920) are performed to separate the roles of
zonally asymmetric aerosol forcings. We find that the WH aerosol forcing,
located in the extratropics, dominates the northward shift of the Hadley cell by inducing an interhemispheric imbalance in radiative forcing. On the other hand, the EH aerosol forcing, located closer to the tropics, dominates the equatorward shift of the NH jet stream. The consistent relationship between the jet stream shift and the top-of-atmosphere net solar flux (FSNTOA) gradient suggests that the latter serves as a rule-of-thumb guidance for the expected shift of the NH jet stream. The surface effect of EH aerosol forcing (mainly from low- to midlatitudes)
is confined more locally and only induces weak warming over the northeastern Pacific and North Atlantic. In contrast, the WH aerosol reduction leads to a large-scale warming over NH mid-to-high latitudes that largely offsets the cooling over the northeastern Pacific due to EH aerosols. The simulated competing roles of regional aerosol forcings in driving
atmospheric circulation and surface temperature responses during the recent
decades highlight the importance of considering zonally asymmetric forcings
(west to east) and also their meridional locations within the NH (tropical
vs. extratropical).