In Situ-Polymerized Separator-Free Ionogel Electrolyte with Enhanced Interfacial Compatibility for Integrated Solid-State Lithium Batteries
Zijie Wei,
Sibin Zhu,
Xiaoming Zhu
et al.
Abstract:The gel polymer electrolyte (GPE) applied in solid lithium metal batteries (LMBs) is often prepared by an ex situ method and subsequently sandwiched between electrodes during battery assembly. However, despite the enhanced ionic conductivity and safety of GPEs, this assembly technique leads to inferior contact between the electrode layer and the electrolyte layer, causing a series of interfacial problems. To address this issue, an innovative in situ polymerization strategy is proposed in this work. First, a so… Show more
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