In Situ Electrochemical Polymerization of Cathode Electrolyte Interphase Enabling High‐Performance Lithium Metal Batteries
Shipeng Sun,
Jiangtao Yu,
Xinyu Ma
et al.
Abstract:Lithium metal batteries (LMBs) with high‐voltage nickel‐rich cathodes show great potential as energy storage devices due to their exceptional capacity and power density. However, the detrimental parasitic side reactions at the cathode electrolyte interface result in rapid capacity decay. Herein, a polymerizable electrolyte additive, pyrrole‐1‐propionic acid (PA), which can be in situ electrochemically polymerized on the cathode surface and involved in forming cathode electrolyte interphase (CEI) film during cy… Show more
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