Bright nitriding of a steel surface is demonstrated by an atmospheric-pressure pulsed-arc plasma jet, keeping the original metallic luster and low roughness. As the hydrogen fraction in the nitrogen-hydrogen gas mixture increases, the optical emission intensity of NH radicals decreases. Following this fact, we examine a method to suppress the formation of a compound layer, in which the hydrogen fraction increases from the conventional value of 1% to larger values for suppressing excess nitrogen supply. The hydrogen fraction of 4% provides a nitrided surface without a compound layer, where surface reflectance is largest and surface roughness is lowest. However, the nitriding treatment produces a dark spot several millimeters in diameter at the sample center due to local oxidization.