Abstract:A B S T R A C TNanometer sized and sheet-like bentonites play an important role in the removal of metal ions from contaminated water. They exist everywhere in nature and can develop a good and less expensive alternative in wastewater cleanup containing heavy metals. However, their use may generate turbid suspensions difficult to settle. Therefore, a coupling of adsorption on natural material was chosen. A modified Algerian bentonite in coagulation/ flocculation processes was used with a biological flocculant o… Show more
“…In the enhanced coagulation process with ferric ions and calcite for high-arsenic water treatment, small arsenic-borne coagulants coating on the calcite surfaces increased the settling rate of the particles (Song et al, 2006). Many different types of particles have been added to aid coagulation performance, including carbon nanotubes (Simate et al, 2012), magnetic particles (MPs) (Zhang et al, 2012), zeolites (Liao et al, 2016), bentonite (Ferhat et al, 2016), silica (Xue et al, 2016), and manganese dioxide (Huangfu et al, 2017). However, these methods not only required large quantities of materials but also produced a considerable amount of sludge, increasing the costs for the subsequent disposal of potentially hazardous sludges.…”
Compositing MPs to AlCl 3 improved primary cluster size and their aggregation. MPs-Al 13 -DOM clusters facilitated DOC removal and residual Al reduction. Significant interaction for turbidity removal was observed between MPs and Al 30 . Interactions between Al species and MPs guide the application of an effective MSC process.
“…In the enhanced coagulation process with ferric ions and calcite for high-arsenic water treatment, small arsenic-borne coagulants coating on the calcite surfaces increased the settling rate of the particles (Song et al, 2006). Many different types of particles have been added to aid coagulation performance, including carbon nanotubes (Simate et al, 2012), magnetic particles (MPs) (Zhang et al, 2012), zeolites (Liao et al, 2016), bentonite (Ferhat et al, 2016), silica (Xue et al, 2016), and manganese dioxide (Huangfu et al, 2017). However, these methods not only required large quantities of materials but also produced a considerable amount of sludge, increasing the costs for the subsequent disposal of potentially hazardous sludges.…”
Compositing MPs to AlCl 3 improved primary cluster size and their aggregation. MPs-Al 13 -DOM clusters facilitated DOC removal and residual Al reduction. Significant interaction for turbidity removal was observed between MPs and Al 30 . Interactions between Al species and MPs guide the application of an effective MSC process.
“…In addition, there are high costs associated with treatment of the concentrate [12]. Traditional flocculants have a poor heavy metal removal capacity and frequently require additional modification or compounding to enhance the removal process [13]. Although adsorption is a relatively traditional processing technique, compared with other technologies, it has the greatest development space and application prospects owing to its low cost, stability, and convenience.…”
Granular-activated carbon is a commonly used adsorbent in water treatment. It can be reused by regeneration when saturated, but there are limits to the number of regenerations in actual engineering. This study created a simple and economical treatment method allowing for the reuse of waste granular-activated carbon (WGAC) that approaches the regeneration limit. The adsorption kinetics, equilibrium, and thermodynamics of Ni(II) onto the treated waste granular-activated carbon (TWGAC) and the new granular-activated carbon (NGAC) were studied. The N 2 adsorption/ desorption isotherms, zeta potential, SEM, energy-dispersive spectrometry and FTIR spectra were used to characterize and compare the NGAC and TWGAC. Analysis revealed that the structure of WGAC was severely damaged, but the adsorption capacity and adsorption mechanism after treatment were similar to those of NGAC. Experimental data showed that the pseudo-second-order kinetic model and the Freundlich isothermal model had high correlation coefficients (R 2 > 0.99). The maximum adsorption capacity of TWGAC and NGAC was 138.9 and 123.5 mg g-1. Thermodynamic parameters, including the negative values ΔG, positive values ΔH, and positive value ΔS, indicated that the current adsorption processes of TWGAC and NGAC were feasible, spontaneous and endothermic. After three cycles, TWGAC's removal rate for Ni(II) remained as high as 95.3%.
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