In Situ Reconstruction of Scalable Amorphous Indium-Based Metal–Organic Framework for CO2 Electroreduction to Formate over an Ultrawide Potential Window
Ziyun Liu,
Xinxin Han,
Junhui Liu
et al.
Abstract:Amorphous
metal–organic frameworks (aMOFs) are highly attractive
for electrocatalytic applications due to their exceptional conductivity
and abundant defect sites, but harsh preparation conditions of “top-down”
strategy have hindered their widespread use. Herein, the scalable
production of aMIL-68(In)-NH2 was successfully achieved
through a facile “bottom-up” strategy involving ligand
competition with 2-methylimidazole. Multiple in situ and ex situ characterizations reveal that aMIL-68(In)-NH2 evolutes into In… Show more
The electrochemical reduction of carbon dioxide (CO 2 RR) to carbon monoxide 11 represents a cost-effective pathway towards realizing carbon neutrality. To suppress 12 the hydrogen evolution reaction (HER), the...
The electrochemical reduction of carbon dioxide (CO 2 RR) to carbon monoxide 11 represents a cost-effective pathway towards realizing carbon neutrality. To suppress 12 the hydrogen evolution reaction (HER), the...
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